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Utilization threshold of surface water and groundwater based on the system optimization of crop planting

Qiang FU,Jiahong LI,Tianxiao LI,Dong LIU,Song CUI

《农业科学与工程前沿（英文）》 2016年 第3卷 第3期   页码 231-240 doi: 10.15302/J-FASE-2016101

摘要： Based on the diversity of the agricultural system, this research calculates the planting structures of rice, maize and soybean considering the optimal economic-social-ecological aspects. Then, based on the uncertainty and randomness of the water resources system, the interval two-stage stochastic programming method, which introduces the uncertainty of the interval number, is used to calculate the groundwater exploitation and the use efficiency of surface water. The method considers the minimum cost of water as the objective of the uncertainty model for surface water and groundwater joint scheduling optimization for different planting structures. Finally, by calculating harmonious entropy, the optimal exploitation utilization interval of surface water and groundwater is determined for optimal cultivation in the Sanjiang Plain. The optimal matching of the planting structure under the economic system is suitable when the mining ratio of the surface is in 44.13%–45.45% and the exploitation utilization of groundwater is in 54.82%–66.86%, the optimal planting structure under the social system is suitable when surface water mining ratio is in 47.84%–48.04% and the groundwater exploitation threshold is in 67.07%–72.00%. This article optimizes the economic-social-ecological-water system, which is important for the development of a water- and food-conserving society and providing a more accurate management environment.

关键词： economic-social-ecological     uncertainty     harmonious entropy     surface water and groundwater     utilization threshold    

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Assessing the impact on groundwater safety of inter-basin water transfer using a coupled modeling approach

Haifeng JIA,Shidong LIANG,Yansong ZHANG

《环境科学与工程前沿（英文）》 2015年 第9卷 第1期   页码 84-95 doi: 10.1007/s11783-014-0741-2

摘要： Surface water and groundwater always behave in a coupled manner and are major components of hydrologic cycle. However, surface water simulation models and groundwater simulation models are run separately most of the time. Few models focus on the impact of hydraulic changes in the surface water flows on the groundwater, or specifically, the impact of a water transfer project to fill a seasonally dry channel. In this study, a linked surface water and groundwater simulation model was developed to assess the impact of a trans-basin water diversion project on the groundwater. A typical plain area east of Beijing was selected as a case study, representing Beijing’s main source of groundwater used for drinking water. A surface water quality model of the Chaobai River was developed based on the Water Quality Analysis Simulation Program (WASP), and a groundwater model was developed based on the Modular Finite-Difference Groundwater Flow Model (MODFLOW) and the Modular 3-D transport model (MT3D). The results of the surface water simulation were used as input for the groundwater simulation. Water levels and four contaminants (NH -N, COD , F, As) were simulated. With the same initial and boundary conditions, scenario analyses were performed to quantify the impact of different quantities of diversion water on the groundwater environment. The results showed the water quality of the groundwater sources was not significantly affected.

关键词： surface water     groundwater     linked model     groundwater safety impact assessment     water diversion    

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The influence of slope collapse on water exchange between a pit lake and a heterogeneous aquifer

Bo Zhang, Xilai Zheng, Tianyuan Zheng, Jia Xin, Shuai Sui, Di Zhang

《环境科学与工程前沿（英文）》 2019年 第13卷 第2期 doi: 10.1007/s11783-019-1104-9

摘要：

Slope collapse will reduce the water exchange.

Slope collapse will affect the spatial distribution of the water exchange.

Precipitation have the most impact on the dynamics of the water exchange.

关键词： Pit lake     Slope collapse     Groundwater–surface water interactions     Numerical simulation    

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Arsenic geochemistry of groundwater in Southeast Asia

Kyoung-Woong Kim, Penradee Chanpiwat, Hoang Thi Hanh, Kongkea Phan, Suthipong Sthiannopkao

《医学前沿（英文）》 2011年 第5卷 第4期   页码 420-433 doi: 10.1007/s11684-011-0158-2

摘要： The occurrence of high concentrations of arsenic in the groundwater of the Southeast Asia region has received much attention in the past decade. This study presents an overview of the arsenic contamination problems in Vietnam, Cambodia, Lao People’s Democratic Republic and Thailand. Most groundwater used as a source of drinking water in rural areas has been found to be contaminated with arsenic exceeding the WHO drinking water guideline of 10 μg·L . With the exception of Thailand, groundwater was found to be contaminated with naturally occurring arsenic in the region. Interestingly, high arsenic concentrations (>10 μg·L ) were generally found in the floodplain areas located along the Mekong River. The source of elevated arsenic concentrations in groundwater is thought to be the release of arsenic from river sediments under highly reducing conditions. In Thailand, arsenic has never been found naturally in groundwater, but originates from tin mining activities. More than 10 million residents in Southeast Asia are estimated to be at risk from consuming arsenic-contaminated groundwater. In Southeast Asia, groundwater has been found to be a significant source of daily inorganic arsenic intake in humans. A positive correlation between groundwater arsenic concentration and arsenic concentration in human hair has been observed in Cambodia and Vietnam. A substantial knowledge gap exists between the epidemiology of arsenicosis and its impact on human health. More collaborative studies particularly on the scope of public health and its epidemiology are needed to conduct to fulfill the knowledge gaps of As as well as to enhance the operational responses to As issue in Southeast Asian countries.

关键词： arsenic     groundwater     drinking water     arsenicosis     Mekong River     Southeast Asia    

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Using hydrochemical signatures to characterize the long-period evolution of groundwater information in

《环境科学与工程前沿（英文）》 2021年 第15卷 第5期 doi: 10.1007/s11783-021-1393-7

摘要：

• The long-period groundwater evolution was identified by hydrochemical signatures.

关键词： Groundwater quality     Hydrochemical signatures     Spatial-temporal variations     Water-rock interactions     Anthropogenic interventions    

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Enhanced photocatalytic water splitting with surface defective SrTiO

Junying LIU, Zhidong WEI, Wenfeng SHANGGUAN

《能源前沿（英文）》 2021年 第15卷 第1期   页码 700-709 doi: 10.1007/s11708-021-0735-2

摘要： Surface reconstructed SrTiO nanocrystals were synthesized by a thermal treatment process in presence of NaBH and SrTiO nanocrystals. The surface reconstruction of SrTiO nanocrystals is attributed to the introduction of surface oxygen vacancies or Ti sites (such as Ti and Ti ) during the hydrogenation treatment process. The light absorption and the charge transfer ability of SrTiO nanocrystals are simultaneously enhanced due to surface oxygen vacancies or Ti sites (such as Ti and Ti ), which are beneficial to photocatalytic water splitting. Meanwhile, these defects also change the redox potential of the photocatalysts. Since there existed a synergistic effect between the three, the ratio of hydrogen to oxygen production was also regulated.

关键词： SrTiO3     surface reconstruction     oxygen vacancies     photocatalytic water splitting    

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Relationships of nitrous oxide fluxes with water quality parameters in free water surface constructed

Juan WU, Jian ZHANG, Wenlin JIA, Huijun XIE, Bo ZHANG

《环境科学与工程前沿（英文）》 2009年 第3卷 第2期   页码 241-247 doi: 10.1007/s11783-009-0023-6

摘要： The effects of chemical oxygen demand (COD) concentration in the influent on nitrous oxide (N O) emissions, together with the relationships between N O and water quality parameters in free water surface constructed wetlands, were investigated with laboratory-scale systems. N O emission and purification performance of wastewater were very strongly dependent on COD concentration in the influent, and the total N O emission in the system with middle COD influent concentration was the least. The relationships between N O and the chemical and physical water quality variables were studied by using principal component scores in multiple linear regression analysis to predict N O flux. The multiple linear regression model against principal components indicated that different water parameters affected N O flux with different COD concentrations in the influent, but nitrate nitrogen affected N O flux in all systems.

关键词： free water surface constructed wetland     nitrous oxide emission     water quality parameter     principal component analysis     multiple linear regression    

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Recent advances in pharmaceuticals and personal care products in the surface water and sediments in China

Wentao Zhao, Ying Guo, Shuguang Lu, Pingping Yan, Qian Sui

《环境科学与工程前沿（英文）》 2016年 第10卷 第6期 doi: 10.1007/s11783-016-0868-4

摘要： Recent publications on PPCPs in surface water environment in China were reviewed. Antibiotics received more attention than other PPCPs in surface water environment. Uneven attention has been focused across different study areas in China. Sulfamethoxazole showed the most significant environmental risk in surface water. Higher risks were posed by PPCPs in sediments than in surface water. Pharmaceuticals and personal care products (PPCPs) have been regarded as an emerging problem in the surface water environment in the past few decades. In China, although related studies were initiated several years ago, an increasing number of studies on this topic have been conducted in recent years. These studies have expanded knowledge of their occurrence, behavior and associated risk in the surface water environment in China. This review compiles the most recent literature related to the studies of PPCPs in the surface water environment in China. It includes PPCP occurrence in surface water and sediments, their geographical distribution, and outcomes of the associated risk assessment. It shows that antibiotics have received much more attention in both surface water and sediments than other PPCPs. Compared to other countries; most antibiotics in the collected sediments in China showed higher contamination levels. Many more study areas have been covered in recent years; however, attention has been given to only specific areas. Environmental risk assessment based on risk quotients indicated that sulfamethoxazole presents the most significant environmental risk to relevant aquatic organisms; followed by ofloxacin, ciprofloxacin, enrofloxacin, 17α-ethynylestradiol, ibuprofen and diclofenac. Despite limited research on the environmental risk assessment of PPCPs in sediments, higher risks posed by PPCPs in the sediments rather than surface water were identified highlighting the need for further risk assessment of PPCPs in sediment samples.

关键词： Surface water     Sediment     Antibiotics     Geographical distribution     Risk assessment    

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Improved nitrogen removal in dual-contaminated surface water by photocatalysis

Yongming ZHANG, Rong YAN, Zhen ZOU, Jiewei WANG, Bruce E. RITTMANN

《环境科学与工程前沿（英文）》 2012年 第6卷 第3期   页码 428-436 doi: 10.1007/s11783-012-0401-3

摘要： River waters in China have dual contamination by nutrients and recalcitrant organic compounds. In principle, the organic compounds could be used to drive denitrification of nitrate, thus arresting eutrophication potential, if the recalcitrant organics could be made bioavailable. This study investigated the potential to make the recalcitrant organics bioavailable through photocatalysis. Batch denitrification tests in a biofilm reactor demonstrated that dual-contaminated river water was short of available electron donor, which resulted in low total nitrogen (TN) removal by denitrification. However, the denitrification rate was increased significantly by adding glucose or by making the organic matters of the river water more bioavailable through photocatalysis. Photocatalysis for 15 min increased the Chemical Oxygen Demand (COD) of the river water from 53 to 84 mg·L and led to a 4-fold increase in TN removal. The increase in TN removal gave the same effect as adding 92 mg·L of glucose. During the photocatalysis experiments, the COD increased because photocatalysis transformed organic molecules from those that are resistant to dichromate oxidation in the COD test to those that can be oxidized by dichromate. This phenomenon was verified by testing photocatalysis of pyridine added to the river water. These findings point to the potential for N removal via denitrification after photocatalysis, and they also suggest that the rivers in China may be far more polluted than indicated by COD assays.

关键词： dual contamination     eutrophication     photocatalysis     remediation     surface water    

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An emerging market for groundwater remediation in China: Policies, statistics, and future outlook

Deyi Hou, Guanghe Li, Paul Nathanail

《环境科学与工程前沿（英文）》 2018年 第12卷 第1期 doi: 10.1007/s11783-018-1027-x

摘要： There is a rapidly emerging and potentially huge market for the remediation of contaminated groundwater in China. The Chinese government published a Water Action Plan in April 2015, a Soil Action Plan in May 2016, and a draft Soil Pollution Prevention and Control Law in June 2017. All of these new policies and regulations put pressures on local governments and contaminated site owners, obliging them to conduct site investigation and to cleanup contaminated groundwater. The Chinese population in northern regions heavily depend on groundwater, with nearly 70% of water supply coming from aquifer sources in the Beijing-Tianjin-Hebei region. However, poor groundwater quality due to natural geochemical background and anthropogeic pollution is a serious concern, with poor or very poor quality water observed in nearly 80% of groundwater monitoring wells in 17 northern provinces. Shallow groundwater in many areas has been contaminated by toxic pollutants such as heavy metals and chlorinated organic compounds. There is an urgent need to better understand the situation and to conduct groundwater remediation at contaminated sites. The Chinese government is investing heavily in the research and development for groundwater remediation, which is expected to greatly add to the quality and quantity of groundwater remediation projects in the near future.

关键词： Groundwater pollution     Contaminated land     Groundwater remediation     Emerging market    

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Catalytic reduction for water treatment

Maocong Hu, Yin Liu, Zhenhua Yao, Liping Ma, Xianqin Wang

《环境科学与工程前沿（英文）》 2018年 第12卷 第1期 doi: 10.1007/s11783-017-0972-0

摘要： Treating water contaminants via heterogeneously catalyzed reduction reaction is a subject of growing interest due to its good activity and superior selectivity compared to conventional technology, yielding products that are non-toxic or substantially less toxic. This article reviews the application of catalytic reduction as a progressive approach to treat different types of contaminants in water, which covers hydrodehalogenation for wastewater treatment and hydrogenation of nitrate/nitrite for groundwater remediation. For hydrodehalogenation, an overview of the existing treatment technologies is provided with an assessment of the advantages of catalytic reduction over the conventional methodologies. Catalyst design for feasible catalytic reactions is considered with a critical analysis of the pertinent literature. For hydrogenation, hydrogenation of nitrate/nitrite contaminants in water is mainly focused. Several important nitrate reduction catalysts are discussed relating to their preparation method and catalytic performance. In addition, novel approach of catalytic reduction using in situ synthesized H evolved from water splitting reaction is illustrated. Finally, the challenges and perspective for the extensive application of catalytic reduction technology in water treatment are discussed. This review provides key information to our community to apply catalytic reduction approach for water treatment.

关键词： Halogenated compounds     Nitrate/nitrite contaminants     Hydrodechloriantion     Hydrogenation     Wastewater treatment     Groundwater remediation    

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Perfluorocarboxylic acids (PFCAs) and perfluoroalkyl sulfonates (PFASs) in surface and tap water around

Yong QIU, He JING, Hanchang SHI,

《环境科学与工程前沿（英文）》 2010年 第4卷 第3期   页码 301-310 doi: 10.1007/s11783-010-0236-8

摘要： Perfluorinated compounds (PFCs) are ubiquitously distributed in the environment mainly as perfluoro-carboxylic acids (PFCAs) and perfluoroalkyl sulfonates (PFASs). In this paper, six PFCAs and two PFASs were quantified in surface and tap water samples from 12 sites around Lake Taihu near Shanghai City in East China. Predominant PFCs were perfluorooctanoic acid (PFOA) and perfluorooctane sulfonate (PFOS), of which the concentration ranges were 6.8–206 and 1.2–45 ng·L, the geometric means were 35.3 and 9.4 ng·L, and the median (quartile range) values were 31.4 (34.4) and 10.4 (10.7) ng·L, respectively. Other PFCs were also detected but in much lower concentrations than PFOA. The sources of the PFCs were expected to be direct industrial discharges in the Lake Taihu area, and this area was also a possible source of PFCs contaminations in Shanghai district in the downstream. PFCs distributions were found different in the upstream, downstream and north part of Lake Taihu. Occurrences of PFCs in the tap water in Lake Taihu area indicated their exposure to the local people. A brief estimation of the environmental risks by PFCs implied no acute or immediate risks from PFCs to local human health, but chronic risks from PFOA in the tap water should be considered in the downstream regions.

关键词： surface and tap water     perfluorocarboxylic acids (PFCAs)     perfluoroalkyl sulfonates (PFASs)     Lake Taihu area     ultra performance liquid chromatography with tandem mass spectrometry (UPLC-MS)    

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Simultaneous removal of arsenate and fluoride from water by Al-Fe (hydr)oxides

Junlian QIAO, Zimin CUI, Yuankui SUN, Qinghai HU, Xiaohong GUAN

《环境科学与工程前沿（英文）》 2014年 第8卷 第2期   页码 169-179 doi: 10.1007/s11783-013-0533-0

摘要： Al-Fe (hydr)oxides with different Al/Fe molar ratios (4∶1, 1∶1, 1∶4, 0∶1) were prepared using a co-precipitation method and were then employed for simultaneous removal of arsenate and fluoride. The 4Al:Fe was superior to other adsorbents for removal of arsenate and fluoride in the pH range of 5.0–9.0. The adsorption capacity of the Al-Fe (hydr)oxides for arsenate and fluoride at pH 6.5±0.3 increased with increasing Al content in the adsorbents. The linear relationship between the amount of OH released from the adsorbent and the amount of arsenate or fluoride adsorbent by 4Al:Fe indicated that the adsorption of arsenate and fluoride by Al-Fe (hydr)oxides was realized primarily through quantitative ligand exchange. Moreover, there was a very good correlation between the surface hydroxyl group densities of Al-Fe (hydr)oxides and their adsorption capacities for arsenate or fluoride. The highest adsorption capacity for arsenate and fluoride by 4Al:Fe is mainly ascribed to its highest surface hydroxyl group density besides its largest pH . The dosage of adsorbent necessary to remove arsenate and fluoride to meet the drinking water standard was mainly determined by the presence of fluoride since fluoride was generally present in groundwater at much higher concentration than arsenate.

关键词： Al-Fe (hydr)oxides     groundwater     adsorption     hydroxyl group     ligand exchange    

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Optimization and modeling of coagulation-flocculation to remove algae and organic matter from surfacewater by response surface methodology

Ziming Zhao, Wenjun Sun, Madhumita B. Ray, Ajay K Ray, Tianyin Huang, Jiabin Chen

《环境科学与工程前沿（英文）》 2019年 第13卷 第5期 doi: 10.1007/s11783-019-1159-7

摘要： Charge neutralization and sweep flocculation were the major mechanisms. Effect of process parameters was investigated. Optimal coagulation conditions were studied by response surface methodology. ANN models presented more robust and accurate prediction than RSM. Seasonal algal blooms of Lake Yangcheng highlight the necessity to develop an effective and optimal water treatment process to enhance the removal of algae and dissolved organic matter (DOM). In the present study, the coagulation performance for the removal of algae, turbidity, dissolved organic carbon (DOC) and ultraviolet absorbance at 254 nm (UV254) was investigated systematically by central composite design (CCD) using response surface methodology (RSM). The regression models were developed to illustrate the relationships between coagulation performance and experimental variables. Analysis of variance (ANOVA) was performed to test the significance of the response surface models. It can be concluded that the major mechanisms of coagulation to remove algae and DOM were charge neutralization and sweep flocculation at a pH range of 4.66–6.34. The optimal coagulation conditions with coagulant dosage of 7.57 mg Al/L, pH of 5.42 and initial algal cell density of 3.83 × 106 cell/mL led to removal of 96.76%, 97.64%, 40.23% and 30.12% in term of cell density, turbidity, DOC and UV254 absorbance, respectively, which were in good agreement with the validation experimental results. A comparison between the modeling results derived through both ANOVA and artificial neural networks (ANN) based on experimental data showed a high correlation coefficient, which indicated that the models were significant and fitted well with experimental results. The results proposed a valuable reference for the treatment of algae-laden surface water in practical application by the optimal coagulation-flocculation process.

关键词： Algae     Coagulation-flocculation     Response surface methodology     Artificial neural networks    

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Simultaneous analysis of five taste and odor compounds in surface water using solid-phase extraction

Wenfeng SUN, Ruibao JIA, Baoyu GAO

《环境科学与工程前沿（英文）》 2012年 第6卷 第1期   页码 66-74 doi: 10.1007/s11783-010-0257-3

摘要： In this paper, a method using solid-phase extraction (SPE) and gas chromatography-mass spectrometry (GC-MS) was developed to simultaneously analyze five taste and odor compounds in surface water, i.e., 2-methylisoborneol (2-MIB), 2,4,6-trichloroanisole (TCA), 2-isopropyl-3-methoxy pyrazine (IPMP), 2-isobutyl-3-methoxy pyrazine (IBMP), and -1,10-dimethyl- -9-decalol (geosmin, GSM). The mass spectrometry was operated in selective ion monitoring (SIM) mode. Three kinds of SPE columns and three eluting solvents were compared, the C18 column was chosen as optimum SPE column, and methanol was chosen as the optimum eluting solvent. It was found that the method showed good linearity in the range of 1–200 ng·L and gave detection limits of 0.5–1.5 ng·L for individual compounds. Good recoveries (93.5%–108%) and relative standard deviations (1.58%–7.31%) were also obtained. Additionally, concentrations of these taste and odor compounds in Jinan’s surface and drinking water were analyzed by applying this method, and the results showed that GSM and 2-MIB were the dominant taste and odor compounds in Jinan’s raw water.

关键词： solid-phase extraction (SPE)     gas chromatography-mass spectrometry (GC-MS)     taste and odor compounds     surface water     micropollutant    

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标题 作者 时间 类型 操作

Utilization threshold of surface water and groundwater based on the system optimization of crop planting

Qiang FU,Jiahong LI,Tianxiao LI,Dong LIU,Song CUI

期刊论文

Assessing the impact on groundwater safety of inter-basin water transfer using a coupled modeling approach

Haifeng JIA,Shidong LIANG,Yansong ZHANG

期刊论文

The influence of slope collapse on water exchange between a pit lake and a heterogeneous aquifer

Bo Zhang, Xilai Zheng, Tianyuan Zheng, Jia Xin, Shuai Sui, Di Zhang

期刊论文

Arsenic geochemistry of groundwater in Southeast Asia

Kyoung-Woong Kim, Penradee Chanpiwat, Hoang Thi Hanh, Kongkea Phan, Suthipong Sthiannopkao

期刊论文

Using hydrochemical signatures to characterize the long-period evolution of groundwater information in

期刊论文

Enhanced photocatalytic water splitting with surface defective SrTiO

Junying LIU, Zhidong WEI, Wenfeng SHANGGUAN

期刊论文

Relationships of nitrous oxide fluxes with water quality parameters in free water surface constructed

Juan WU, Jian ZHANG, Wenlin JIA, Huijun XIE, Bo ZHANG

期刊论文

Recent advances in pharmaceuticals and personal care products in the surface water and sediments in China

Wentao Zhao, Ying Guo, Shuguang Lu, Pingping Yan, Qian Sui

期刊论文

Improved nitrogen removal in dual-contaminated surface water by photocatalysis

Yongming ZHANG, Rong YAN, Zhen ZOU, Jiewei WANG, Bruce E. RITTMANN

期刊论文

An emerging market for groundwater remediation in China: Policies, statistics, and future outlook

Deyi Hou, Guanghe Li, Paul Nathanail

期刊论文

Catalytic reduction for water treatment

Maocong Hu, Yin Liu, Zhenhua Yao, Liping Ma, Xianqin Wang

期刊论文

Perfluorocarboxylic acids (PFCAs) and perfluoroalkyl sulfonates (PFASs) in surface and tap water around

Yong QIU, He JING, Hanchang SHI,

期刊论文

Simultaneous removal of arsenate and fluoride from water by Al-Fe (hydr)oxides

Junlian QIAO, Zimin CUI, Yuankui SUN, Qinghai HU, Xiaohong GUAN

期刊论文

Optimization and modeling of coagulation-flocculation to remove algae and organic matter from surfacewater by response surface methodology

Ziming Zhao, Wenjun Sun, Madhumita B. Ray, Ajay K Ray, Tianyin Huang, Jiabin Chen

期刊论文

Simultaneous analysis of five taste and odor compounds in surface water using solid-phase extraction

Wenfeng SUN, Ruibao JIA, Baoyu GAO

期刊论文